I have two simple suggestions for the Sample Recorder dialog:
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An additional option for “sync start & stop”: sync to beat (and maybe to line), so that recording starts on the next beat (or line). This would make it easy to record a sample synced to the song without the need to wait for the next pattern to play. This would be especially cool combined with something like this.
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An additional option to create a new sample within the same instrument on each take. I’d find this more useful than the “create a new instrument on each take” option (though that option should also be available, of course).